Get Advances in Electrochemical Science and Engineering, Volume PDF

By Richard C. Alkire, Charles W. Tobias

ISBN-10: 352729385X

ISBN-13: 9783527293858

ISBN-10: 3527616799

ISBN-13: 9783527616794

ISBN-10: 3527616888

ISBN-13: 9783527616886

This sequence, previously edited through Heinz Gerischer and Charls V. Tobias, now edited via Richard C. Alkire and Dieter M. Kolb, has been warmly welcomed through scientists world-wide that's mirrored within the stories of the former volumes:

'This is an important booklet for researchers in electrochemistry; it covers parts of either primary and functional value, with stories of top quality. the fabric is especially good awarded and the alternative of issues displays a balanced editorial coverage that's welcomed.' The Analyst

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Extra resources for Advances in Electrochemical Science and Engineering, Volume 5

Sample text

Similar values are obtained from the calculation according to Eq. (6). 38 eV in N,N-dimethylformamide solutions has been found in [ 1301 for electron exchange between anthracene and its radical anion). These calculations must be treated only as a semiquantitative approach until the systematic temperature study of efficiency has been done, especially as the DPA ECL system has been studied only in a limited number of solvents. As mentioned above, the ECL system containing rubrene is somewhat more complicated, but has been studied in more detail.

11. 10-diphenylanthracene (B). Potential energy curves are presented in the zero-order approximation, without removing the degeneracy at the crossing points of the potential energy curves. Broken lines represent the vibronically excited triplet state. converted in primary TTA may also take part in the triplet-triplet annihilation (real bimolecular, secondary TTA according to reaction (37)). Such a process leads, however, to much less efficient formation of the excited singlet states. The ECL efficiencies $eel reported for both hydrocarbons are fairly large (up to a few percent), at least an order of magnitude greater than those found for ECL processes occurring according to a “pure” T-route.

45) unimolecular reaction rates are introduced. They arise from the assumption of similar structures of the precursor complex for all three reaction channels, which seems to be allowed in the view of the minimum energy and maximum orbital overlap rules. The reaction rate, k3, corresponding to population of the excited triplet, is multiplied by the statistical factor relating to spin multiplicity. The reaction mechanism of excited singlet formation in rubrene ECL seems to be a superposition of two parallel processes.

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Advances in Electrochemical Science and Engineering, Volume 5 by Richard C. Alkire, Charles W. Tobias


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